We review an iconic class of chemical oscillators driven by phase transition instabilities, namely Gas Evolution Oscillators (GEOs). These systems show oscillatory dynamics in the delivery of gas sustained simple reactions yielding gaseous products in a liquid mixture, due to nucleation and supersaturation phenomena. After presenting the main features and properties of these systems, we deepen the underlying mechanism through a unified picture of the various models that have been proposed to describe this kind of oscillations. We finally discuss a concrete example of how such instabilities can impact chemical processes with applied relevance.

Budroni, M.A., Rustici, M., Rossi, F. (2024). Exploring Gas Evolution Oscillators: Mechanisms and Applications. CHEMPHYSCHEM [10.1002/cphc.202400841].

Exploring Gas Evolution Oscillators: Mechanisms and Applications

Budroni, Marcello A.;Rossi, Federico
2024-01-01

Abstract

We review an iconic class of chemical oscillators driven by phase transition instabilities, namely Gas Evolution Oscillators (GEOs). These systems show oscillatory dynamics in the delivery of gas sustained simple reactions yielding gaseous products in a liquid mixture, due to nucleation and supersaturation phenomena. After presenting the main features and properties of these systems, we deepen the underlying mechanism through a unified picture of the various models that have been proposed to describe this kind of oscillations. We finally discuss a concrete example of how such instabilities can impact chemical processes with applied relevance.
2024
Budroni, M.A., Rustici, M., Rossi, F. (2024). Exploring Gas Evolution Oscillators: Mechanisms and Applications. CHEMPHYSCHEM [10.1002/cphc.202400841].
File in questo prodotto:
File Dimensione Formato  
ChemPhysChem - 2024 - Budroni - Exploring Gas Evolution Oscillators Mechanisms and Applications.pdf

accesso aperto

Tipologia: PDF editoriale
Licenza: Creative commons
Dimensione 2.24 MB
Formato Adobe PDF
2.24 MB Adobe PDF Visualizza/Apri

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11365/1280597